Though sulfamethoxazole (SMX) degradation at the low or medium concentration (SMX less then 30 mg/L) has been reported in the microbial fuel cell (MFC), further exploration is still urgently required to investigate how the high concentration of SMX affect the anode biofilm formation. In this study, the degradation mechanism of SMX and the response of microbial community to SMX at different initial concentrations (0, 0.5, 5 and 50 mg/L) were investigated in MFCs. The highest SMX removal efficiency of 98.4% was obtained in MFC (5 mg/L). SMX at optimal concentration (5 mg/L) could serve as substrate accelerating the extracellular electron transfer. However, high concentration of SMX (50 mg/L) conferred significant inhibition on the electron transfer with SMX removal decline to 84.4%. The 16S rRNA high-throughput sequencing revealed the significant shift of the anode biofilms communities with different initial SMX concentrations were observed in MFCs. Thauera and Geobacter were the predominant genus, with relative abundance of 31.9% in MFC (50 mg/L SMX) and 52.7% in MFC (5 mg/L SMX). Methylophilus exhibited a huge increase with the highest percentage of 16.4% in MFC (50 mg/L). Hence, the functional bacteria of Thauera, Geobacter and Methylophilus endowed significant tolerance to the selection pressure from high concentration of SMX in MFCs. Meanwhile, some bacteria including Ornatilinea, Dechloromonas and Longilinea exhibited a decrease or even disappeared in MFCs. Therefore, initial concentrations of SMX played a fundamental role in modifying the relative abundance of predominant populations. This finding would promote theories support for understanding the evolution of anode biofilm formation related to the different initial concentrations of SMX in MFCs.The recovery of uranium from wastewater and safe treatment of U(VI)-containing wastewater are of great important to ensure the sustainable development of nuclear-related energy. Although abundant studies of U(VI) sorption on various adsorbents have been widely achieved, U(VI) sorption at extreme pH and trace concentration is challenging issues due to limited sorption activity of natural adsorbents. The development of novel materials with highly efficient and excellent selectivity for capturing U(VI) from nuclear-related wastewater and seawater is highly desirable. In this study, amidoxime/carbon nitride (AO/g-C3N4) was fabricated and captured U(VI) under a variety of water chemistry. We demonstrated that AO/g-C3N4 exhibited the high adsorption capacities (312 mg/g at pH 6.8), fast removal equilibrium (>98% at 10 min) and superior selectivity for U(VI) compared with the other radionuclides (e.g., 19.76 mg/g of Cs(I)). In addition, AO/g-C3N4 exhibited the high uranium extraction capacity from natural seawater (9.55 mg/g at saturation time of 5.5 days) compared to vanadium (1.85 mg/g). U(VI) adsorption behavior at different pH can be excellently fitted by the surface complexation modeling with three inner sphere surface complexes (i.e., SOUO2(CO3)23-, SO(UO2)3(OH)50 and SOUO2+ species). According to XPS (X-ray Photoelectron Spectroscopy) analysis, the strong complexation of U(VI) with AO groups retained in C3N4 nanosheet. The split of U-Oeq2 subshell and the occurrence of U-C shell further demonstrated inner-sphere surface complexation by EXAFS (X-Ray Absorption Fine Structure) spectra analyses. These results revealed that the high potential of AO/g-C3N4 materials for selective U(VI) capture from wastewater and seawater.The co-presence of arsenic (As) and antimony (Sb) in water bodies has been commonly reported. The toxicity of As and Sb varies with different speciation. Herein, we designed a dual-functional electrochemical filter toward "one-step" detoxification and sequestration of highly toxic As(III) and Sb(III). The key to this technology is a functional anodic filter consists of nanoscale goethite and carbon nanotubes (CNT). Results showed that 97.9% As(III) and 91.9% Sb(III) transformation and 86.4% Astotal and 70.1% Sbtotal removal efficiency can be obtained over 2 h continuous filtration under optimized conditions. The Astotal removal kinetics and efficiency enhanced with flow rate and applied voltage (e.g., the Astotal removal efficiency increased from 62.9% at 0 V to 86.4% at 2.5 V). This enhancement in kinetics and efficiency can be explained by the synergistic effects of the flow-through design, plentiful exposed sorption sites, electrochemical reactivity, and nanoscale goethite. Moreover, the proposed technology works effectively across a wide pH range. https://www.selleckchem.com/products/gpr84-antagonist-8.html Only negligible inhibition was observed in the presence of nitrate, chloride, and carbonate. Exhausted hybrid filters can be effectively regenerated by using chemical wash with NaOH solution. This study not only revealed the different adsorption behaviors of As(III) and Sb(III) on the hybrid filters, but also provided new insights into rational design of continuous-flow filters toward simultaneous decontamination of As(III) and Sb(III).The anaerobic co-digestion (coAD) of swine manure (SM) and rice straw (RS) is appealing for renewable energy recovery and waste treatment worldwidely. Improving its performance is very important for its application. In this study, long-term semi-continuous experiments were conducted to evaluate the improving effects of digestate recirculation on the performance, energy recovery, and microbial community of two-stage thermophilic-mesophilic coAD of swine manure (SM) and rice straw (RS). The experimental results indicated that the coAD systems of SM and RS (mixing ratio of 31) with or without digestate recirculation could not realize phase separation. The reactors of both coAD systems were characterized by pH values ranging from 7.74 to 7.85, methane production as 0.41 ± 0.02 and 0.44 ± 0.03 L/L/d, and stable operation. Notably, digestate recirculation increased total methane production, organic matter removal, and reaction rate of the coAD system by 9.92 ± 5.08, 5.22 ± 1.94, and 9.73-12.60%, respectively. Digestate recirculation improved the performance of the coAD by significantly increasing the abundance of Methanosarcina (from 4.1% to 7.5%-10.7% and 35.7%) and decreasing that of Methanothermobacter (from 94.2% to 87.3%-83.6% and 56.8%). Thus, the main methanogenesis pathway of the coAD system was changed by digestate recirculation and the methane production was effectively improved. Although the energy input of the coAD system increased by 30.26%, digestate recirculation improved the energy balance of the total system by 6.83%.